Engineering of benzoxazinoid biosynthesis in Arabidopsis thaliana: Metabolic and physiological challenges
Author
Abramov, Aleksej
* & Chair of Plant Breeding, Technical University of Munich, Liesel-Beckman Str. 2, 85354, Freising, Germany
Author
Hoffmann, Thomas
Author
Stark, Timo D.
Author
Zheng, Linlin
Author
Lenk, Stefan
Author
Hammerl, Richard
Author
Lanzl, Tobias
Author
Dawid, Corinna
Author
Schon, Chris-Carolin
Author
Schwab, Wilfried
Author
Gierl, Alfons
Author
Frey, Monika
text
Phytochemistry
2021
112947
2021-12-31
192
1
15
http://dx.doi.org/10.1016/j.phytochem.2021.112947
journal article
10.1016/j.phytochem.2021.112947
1873-3700
5.9. Isolation of
Arabidopsis
microsomes and P450 assay
15 g
of rosette leaves of 28 dag
Arabidopsis
plants were ground in 200 mL extraction buffer (100 mM ascorbic acid, 1 mM EDTA, 100 mM Tris, 20% v/v glycerol, 20% w/v Sucrose, 5 mM Dithiothreitol) with
4.5 g
Polyklar AT (Merck) and sea sand. The raw extract was filtered through cloth and centrifuged twice at 15 000 g for 10 min. Microsomes were isolated from the supernatant by centrifugation at 120 000
g
for 40 min and resuspended in 1 mL suspension buffer (50 mM potassium phosphate buffer pH 7.5, 20% v/v Glycerol, 1 mM Dithiothreitol). The integrity of the microsomes was tested by measuring the cytochrome C reductase activity as described by
Urban et al. (1990)
.
The
in vitro
activity of the BX P450 enzymes was tested by incubation of
1 mg
total microsomal protein with the respective substrate (2 mM Indole, 1 mM
ION
, 250 μM HION, 200 μM HBOA) in 100 mM potassium phosphate buffer pH 7.5 and 1 mM NADPH at room temperature. The reaction was stopped after 30 min by addition of 1 vol methanol and precipitated protein was pelleted by centrifugation. 2.5 vol of 100 mM acetic acid were added to the supernatant and the products were extracted three times with 2 vol of ethyl acetate. The solvent was evaporated in a vacuum centrifuge, the remaining products were resolved in methanol and analysed by HPLC.